Water Column Methods
We had the opportunity to collect
water column data during six 4-day cruises aboard the R.V. Pelican that
bracketed low and high river discharge conditions (Fig. 1). The corresponding cruise dates were: October
19-22, November 20-23,

Fig. 1:
Sample collection and on-board
analysis of samples was a 24 hour a day process that required a coordinated
effort from everyone in the research group.
The goals of our sampling lay-out and cruise schedule was to obtain a
water column inventory of 222Rn, to collect cores to analyze porewaters for 222Rn and 223Ra/224Ra,
and to collect 4He/3He/3H samples for tracer
and groundwater age data. The CTD
rosette consists of 12-20 L cylinders that are independently fired at specific
depths in the water column. 222Rn
samples were collected by transferring water from the CTD rosette into a 6 L
bottle that was immediately sealed to prevent gas loss. The samples were then analyzed in the
on-board radon lab using a technique similar to Mathieu et al. (1988). This technique consists of sparging the sample with helium and collecting 222Rn
in a trap at liquid nitrogen temperature.
The 222Rn is then transferred to a Lucas cell and counted
with a photomultiplier tube. Porewater 222Rn samples were collected by
weighing a specific section of the core and transferring it into a 6 L bottle
that was pre-filled with 6 L of radon-free water and analyzed as described
above. Porewater
radium isotopes were collected from box cores and Kasten
cores that were centrifuged on-board and the pore fluids were collected and
analyzed at

Mike standing beside the CTD rosette. Dail holding a core that was subsampled from
the box core.

Clay
collecting a sediment sample for porewater
222Rn. The on-board radon lab.
Extraction lines to the left and
counters in the background.

Dan, Erin, Clay, and Reide sampling a core using an
extruder. The on-board centrifuge was used to extract pore
fluids for
radium isotope analysis.

Brion, Kat, and